Background
N-glycolylneuraminic acid (Neu5Gc) is an aberrant glycosylation found in human tumour cells and has been proposed as a cancer biomarker. Until our recent work, no progress has been made towards the development of a Neu5Gc biomarker-based assay for cancer detection and monitoring. Using our purpose-engineered Neu5Gc-specific, lectin, SubB2M, we detected elevated Neu5Gc in sera from ovarian cancer patients. Here we use SubB2M to detect Neu5Gc tumour biomarkers in sera from breast cancer patients.
Methods
Using a surface plasmon resonance (SPR)-based assay with SubB2M for detection, we analyzed serum samples from 96 patients with Stage I - IV breast cancer, as well as 22 cancer-free controls. In addition, we analyzed serum samples from a cohort of patients with high-risk breast cancer collected prospectively over time.
Results
Significantly elevated mean levels of Neu5Gc glycans were detected in serum from patients with all stages of breast cancer compared to cancer-free controls (P value = <0.0001 for all stages). Receiver operating characteristic analyses showed that serum Neu5Gc levels can discriminate Stage I patients from cancer-free individuals with 95.83% sensitivity and 100% specificity, while Stage II, Stage III and Stage IV patients can be distinguished from cancer-free individuals with 100% sensitivity and 100% specificity. Analysis of a series of serum samples collected prospectively, post-diagnosis from a cohort of high-risk breast cancer patients showed a trend for a decrease in Neu5Gc levels immediately following treatment.
Conclusions
Detection of Neu5Gc-glycans using SubB2M may be useful for early detection of breast cancer and as a tool for monitoring treatment and progression in late stage disease.
Impact
A blood-based biomarker test for early detection and accurate monitoring of disease progression in breast cancer would drastically improve patient outcomes.